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Sustainable Synaptic Device with Two‐Dimensional Ferroelectric Materials for Neuromorphic Computing

Source: PubMed Central Open Access, NCBI / U.S. National Library of Medicine

Advanced ScienceLast synced 7/23/2026Status: syncedPMID: 42095516 pmidDOI: 10.1002/advs.202600064

ABSTRACT To overcome the coming big‐data era, significant efforts are needed to implement neuromorphic computing that mimics the functional and structural features of the human brain using electronic devices. Repeated updates mimicking biological synaptic plasticity degrade the endurance of synaptic devices during in situ training. This study demonstrates a two‐dimensional (2D) ferroelectric α‐InSe‐based synaptic device with enhanced durability via self‐curing performed from current annealing (CA) in synaptic fatigue occurring during repetitive learning. The conduction, degradation, and self‐curing mechanisms of the 2D ferroelectric‐based synaptic device are quantitatively elucidated by low‐frequency noise (LFN) spectroscopy. The classification accuracy of the Canadian Institute for Advanced Research (CIFAR)‐10 dataset with self‐cured conductance is superior to that of the device with synaptic fatigue and recovers to the initial accuracy level. The simulation results of removing defect cells through self‐curing in the 2D ferroelectric synaptic array can help reduce energy consumption in the long term. The experimental results emphasize adopting 2D ferroelectric materials for future neuromorphic computing. α‐InSebased FeSFETs can be utilized as sustainable devices through polarization switching governed by both out‐of‐plane and in‐plane polarizations. Upon reaching a fatigued state, current annealing enabled by conductance modulation can significantly enhance the endurance of

Abstract

ABSTRACT To overcome the coming big‐data era, significant efforts are needed to implement neuromorphic computing that mimics the functional and structural features of the human brain using electronic devices. Repeated updates mimicking biological synaptic plasticity degrade the endurance of synaptic devices during in situ training. This study demonstrates a two‐dimensional (2D) ferroelectric α‐InSe‐based synaptic device with enhanced durability via self‐curing performed from current annealing (CA) in synaptic fatigue occurring during repetitive learning. The conduction, degradation, and self‐curing mechanisms of the 2D ferroelectric‐based synaptic device are quantitatively elucidated by low‐frequency noise (LFN) spectroscopy. The classification accuracy of the Canadian Institute for Advanced Research (CIFAR)‐10 dataset with self‐cured conductance is superior to that of the device with synaptic fatigue and recovers to the initial accuracy level. The simulation results of removing defect cells through self‐curing in the 2D ferroelectric synaptic array can help reduce energy consumption in the long term. The experimental results emphasize adopting 2D ferroelectric materials for future neuromorphic computing. α‐InSebased FeSFETs can be utilized as sustainable devices through polarization switching governed by both out‐of‐plane and in‐plane polarizations. Upon reaching a fatigued state, current annealing enabled by conductance modulation can significantly enhance the endurance of FeSFETs. Moreover, current annealing can be selectively and dynamically applied to defective cells in real time at the system level, while maintaining a desirable and optimized power consumption. advs75511-abs-0001 graphical

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